CAS OpenIR
Constructing single Cu-N-3 sites for CO2 electrochemical reduction over a wide potential range
Feng, Jiaqi1,2; Zheng, Lirong3; Jiang, Chongyang1,2; Chen, Zhipeng4; Liu, Lei1; Zeng, Shaojuan1; Bai, Lu1; Zhang, Suojiang1,2; Zhang, Xiangping1,2
2021-06-30
Source PublicationGREEN CHEMISTRY
ISSN1463-9262
Pages6
AbstractA Cu-N-doped carbon nanotube with an unsaturated coordination Cu atom (Cu-N-3) was fabricated and it exhibited over 90% CO faradaic efficiency (FE) in a wide potential range from -0.42 to -0.92 V. The maximum CO FE can reach 98.7% with a high CO partial current density of 234.3 mA cm(-2) in a flow cell. Theoretical calculations elucidated that the Cu-N-3 site facilitated the formation of COOH*, thereby accelerating the CO2 electrochemical reduction.
DOI10.1039/d1gc01914g
Language英语
WOS KeywordEFFICIENT CO2 ; IONIC LIQUIDS ; ELECTROREDUCTION ; CATALYSTS
Funding ProjectNational Key R&D Program of China[2018YFB0605802] ; National Natural Science Foundation of China[21838010] ; National Natural Science Foundation of China[21890762] ; National Natural Science Foundation of China[21921005] ; Key Research Program of Chinese Academy of Science[ZDRW-ZS-2018-1-3] ; Program of Beijing Municipal Natural Science Foundation[2182071] ; International Partnership Program of Chinese Academy of Sciences[122111KYSB20190029] ; Instrument Developing Project of the Chinese Academy of Sciences[YJKYYQ20200062]
WOS Research AreaChemistry ; Science & Technology - Other Topics
WOS SubjectChemistry, Multidisciplinary ; Green & Sustainable Science & Technology
Funding OrganizationNational Key R&D Program of China ; National Natural Science Foundation of China ; Key Research Program of Chinese Academy of Science ; Program of Beijing Municipal Natural Science Foundation ; International Partnership Program of Chinese Academy of Sciences ; Instrument Developing Project of the Chinese Academy of Sciences
WOS IDWOS:000674761500001
PublisherROYAL SOC CHEMISTRY
Citation statistics
Document Type期刊论文
Identifierhttp://ir.ipe.ac.cn/handle/122111/49475
Collection中国科学院过程工程研究所
Corresponding AuthorZhang, Suojiang; Zhang, Xiangping
Affiliation1.Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiphase Complex Syst, Beijing Key Lab Ion Liquids Clean Proc, Beijing 100190, Peoples R China
2.Univ Chinese Acad Sci, Coll Chem Engn, Beijing 100190, Peoples R China
3.Chinese Acad Sci, Inst High Energy Phys, Beijing Synchrotron Radiat Facil BSRF, Beijing 100190, Peoples R China
4.Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, CAS Key Lab Biobased Mat, Qingdao 266101, Peoples R China
Recommended Citation
GB/T 7714
Feng, Jiaqi,Zheng, Lirong,Jiang, Chongyang,et al. Constructing single Cu-N-3 sites for CO2 electrochemical reduction over a wide potential range[J]. GREEN CHEMISTRY,2021:6.
APA Feng, Jiaqi.,Zheng, Lirong.,Jiang, Chongyang.,Chen, Zhipeng.,Liu, Lei.,...&Zhang, Xiangping.(2021).Constructing single Cu-N-3 sites for CO2 electrochemical reduction over a wide potential range.GREEN CHEMISTRY,6.
MLA Feng, Jiaqi,et al."Constructing single Cu-N-3 sites for CO2 electrochemical reduction over a wide potential range".GREEN CHEMISTRY (2021):6.
Files in This Item:
There are no files associated with this item.
Related Services
Recommend this item
Bookmark
Usage statistics
Export to Endnote
Google Scholar
Similar articles in Google Scholar
[Feng, Jiaqi]'s Articles
[Zheng, Lirong]'s Articles
[Jiang, Chongyang]'s Articles
Baidu academic
Similar articles in Baidu academic
[Feng, Jiaqi]'s Articles
[Zheng, Lirong]'s Articles
[Jiang, Chongyang]'s Articles
Bing Scholar
Similar articles in Bing Scholar
[Feng, Jiaqi]'s Articles
[Zheng, Lirong]'s Articles
[Jiang, Chongyang]'s Articles
Terms of Use
No data!
Social Bookmark/Share
All comments (0)
No comment.
 

Items in the repository are protected by copyright, with all rights reserved, unless otherwise indicated.