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Heteroatoms in graphdiyne for catalytic and energy-related applications
Liu, Baokun1,2; Xu, Lekai3; Zhao, Yasong3; Du, Jiang1,2; Yang, Nailiang3,4; Wang, Dan3,4
2021-07-13
Source PublicationJOURNAL OF MATERIALS CHEMISTRY A
ISSN2050-7488
Pages19
AbstractThe recently discovered carbon allotrope GDY possesses rich acetylenic bonds and unique pore structures, prompting GDY as an ideal candidate, tuning its electronic structure by introducing heteroatoms, broadening its usage in catalysis, energy storage and other fields. In this paper, we review different approaches to introduce heteroatoms into GDYs, including monodoping and co-doping, predesigned bottom-up synthesis of GDY, the anchoring of metal atoms into GDYs. Furthermore, we introduce the electronic properties' modification caused by these heteroatoms, including reduced diffusion barrier and adsorption energy, abundant active sites, high reversible capacity and cyclic stability, better rate performance and longer lifespan. Furthermore, the topological molecular structure of GDYs can be tuned through bottom-up synthesis methods with different monomers. GDY has great prospects for inclusion in energy storage devices such as sodium-ion batteries, lithium-ion batteries, lithium/magnesium sulfur batteries, and in electrocatalytic processes such as hydrogen evolution reactions, oxygen reduction reactions, and electrocatalytic nitrogen reduction reactions in important industrial reactions. At the end of this review, challenges and prospects of heteroatoms' introduction into GDY are discussed.
DOI10.1039/d1ta03634c
Language英语
WOS KeywordNITROGEN-DOPED GRAPHDIYNE ; OXYGEN-REDUCTION REACTION ; METAL-FREE CATALYSTS ; LITHIUM-ION ; HIGH-CAPACITY ; INTERFACIAL SYNTHESIS ; CARBON NANOTUBES ; ANODE MATERIAL ; CO OXIDATION ; GRAPHENE
WOS Research AreaChemistry ; Energy & Fuels ; Materials Science
WOS SubjectChemistry, Physical ; Energy & Fuels ; Materials Science, Multidisciplinary
WOS IDWOS:000680401400001
PublisherROYAL SOC CHEMISTRY
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Document Type期刊论文
Identifierhttp://ir.ipe.ac.cn/handle/122111/49497
Collection中国科学院过程工程研究所
Corresponding AuthorDu, Jiang; Yang, Nailiang; Wang, Dan
Affiliation1.Zhengzhou Univ, Sch Mat Sci & Engn, Henan Prov Ind Technol Res Inst Resources & Mat, Zhengzhou 450001, Peoples R China
2.Zhengzhou Univ, Coll Chem, Green Catalysis Ctr, Zhengzhou 450000, Peoples R China
3.Chinese Acad Sci, Inst Proc Engn, State Key Lab Biochem Engn, 1 Beiertiao, Beijing 100190, Peoples R China
4.Univ Chinese Acad Sci, 19A Yuquan Rd, Beijing 100049, Peoples R China
Recommended Citation
GB/T 7714
Liu, Baokun,Xu, Lekai,Zhao, Yasong,et al. Heteroatoms in graphdiyne for catalytic and energy-related applications[J]. JOURNAL OF MATERIALS CHEMISTRY A,2021:19.
APA Liu, Baokun,Xu, Lekai,Zhao, Yasong,Du, Jiang,Yang, Nailiang,&Wang, Dan.(2021).Heteroatoms in graphdiyne for catalytic and energy-related applications.JOURNAL OF MATERIALS CHEMISTRY A,19.
MLA Liu, Baokun,et al."Heteroatoms in graphdiyne for catalytic and energy-related applications".JOURNAL OF MATERIALS CHEMISTRY A (2021):19.
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