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Highly Dispersed Cu/Graphene Nanocatalyst Guided by MOF Structure: Application to Methanol Synthesis from CO2 Hydrogenation
San, Xiaoguang1; Gong, Xiaohui1; Hu, Yanbing2; Hu, Yue3; Wang, Guosheng1; Qi, Jian4; Meng, Dan1; Jin, Quan3
2021-06-28
Source PublicationCHEMISTRYSELECT
ISSN2365-6549
Volume6Issue:24Pages:6115-6118
AbstractThe dispersion of heterogeneous catalyst is directly related to the performance. In this work, highly dispersed Cu/graphene catalyst was successfully prepared by adopting a "template genetic inheritance" (TGI). The metal-organic frameworks (MOFs) were introduced between the graphene sheets. Due to the spatial structure of MOFs, the Cu atoms arranged in the expected direction after removing the MOFs skeleton, which lead to a highly orderly dispersion of the Cu particles with uniform sized. Meanwhile, graphene provided a large specific surface area and a carbon source for in-situ reduction of CuO. Furthermore, the CO2 hydrogenation to methanol performance was analyzed and more than 22 % conversion of CO2 and 84 % selectivity of methanol was achieved. This work provides a simple and novel strategy for the preparation of highly dispersed metal particle supported catalysts, which may be used in catalysis and other fields.
KeywordCO2 hydrogenation graphene methanol synthesis MOFs
DOI10.1002/slct.202101179
Language英语
WOS KeywordCARBON-DIOXIDE ; CATALYST
Funding ProjectNational Natural Science Foundation of China[61973223] ; National Natural Science Foundation of China[51672276] ; National Natural Science Foundation of China[51772294] ; National Natural Science Foundation of China[51972306] ; Liaoning Educational Department Foundation[LQ2019013] ; Liaoning Provincial Natural Science Foundation[2019-ZD-0072] ; Liaoning Revitalization Talents Program[XLYC2007051]
WOS Research AreaChemistry
WOS SubjectChemistry, Multidisciplinary
Funding OrganizationNational Natural Science Foundation of China ; Liaoning Educational Department Foundation ; Liaoning Provincial Natural Science Foundation ; Liaoning Revitalization Talents Program
WOS IDWOS:000674320500035
PublisherWILEY-V C H VERLAG GMBH
Citation statistics
Document Type期刊论文
Identifierhttp://ir.ipe.ac.cn/handle/122111/49540
Collection中国科学院过程工程研究所
Corresponding AuthorMeng, Dan; Jin, Quan
Affiliation1.Shenyang Univ Chem Technol, Coll Chem Engn, 11th St, Shenyang 110142, Peoples R China
2.Jilin Univ, Hosp 2, 218 Zigiang St, Changchun 130021, Peoples R China
3.Jilin Univ, Sch Mat Sci & Engn, Minist Educ, Key Lab Automobile Mat, 5988 Renmin St, Changchun 130022, Peoples R China
4.Chinese Acad Sci, Inst Proc Engn, State Key Lab Biochem Engn, 1 North 2nd St, Beijing 100190, Peoples R China
Recommended Citation
GB/T 7714
San, Xiaoguang,Gong, Xiaohui,Hu, Yanbing,et al. Highly Dispersed Cu/Graphene Nanocatalyst Guided by MOF Structure: Application to Methanol Synthesis from CO2 Hydrogenation[J]. CHEMISTRYSELECT,2021,6(24):6115-6118.
APA San, Xiaoguang.,Gong, Xiaohui.,Hu, Yanbing.,Hu, Yue.,Wang, Guosheng.,...&Jin, Quan.(2021).Highly Dispersed Cu/Graphene Nanocatalyst Guided by MOF Structure: Application to Methanol Synthesis from CO2 Hydrogenation.CHEMISTRYSELECT,6(24),6115-6118.
MLA San, Xiaoguang,et al."Highly Dispersed Cu/Graphene Nanocatalyst Guided by MOF Structure: Application to Methanol Synthesis from CO2 Hydrogenation".CHEMISTRYSELECT 6.24(2021):6115-6118.
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