CAS OpenIR
Enzyme-photo-coupled catalytic systems
Zhang, Shaohua2,6; Liu, Shusong1; Sun, Yiying2; Li, Shihao2; Shi, Jiafu1,4,5; Jiang, Zhongyi2,3,4
2021-11-04
Source PublicationCHEMICAL SOCIETY REVIEWS
ISSN0306-0012
Pages18
AbstractEfficient chemical transformation in a green, low-carbon way is crucial for the sustainable development of modern society. Enzyme-photo-coupled catalytic systems (EPCS) that integrate the exceptional selectivity of enzyme catalysis and the unique reactivity of photocatalysis hold great promise in solar-driven 'molecular editing'. However, the involvement of multiple components and catalytic processes challenged the design of efficient and stable EPCS. To show a clear picture of the complex catalytic system, in this review, we analyze EPCS from the perspective of system engineering. First, we disintegrate the complex system into four elementary components, and reorganize these components into biocatalytic and photocatalytic ensembles (BE and PE). By resolving current accessible systems, we identify that connectivity and compatibility between BE and PE are two crucial factors that govern the performance of EPCS. Then, we discuss the origin of undesirable connectivity and low compatibility, and deduce the possible solutions. Based on these understandings, we propose the designing principles of EPCS. Lastly, we provide a future perspective of EPCS.
DOI10.1039/d1cs00392e
Language英语
WOS KeywordCARBON-DIOXIDE ; REDUCTION ; OXIDATION ; CO2
Funding ProjectNational Key Research and Development Program of China[2020YFA0907902] ; National Natural Science Funds of China[21776213] ; National Natural Science Funds of China[21621004] ; Natural Science Fund of Tianjin[19JCYBJC19700] ; Open Funding Project of the State Key Laboratory of Biochemical Engineering[2020KF-06] ; Tianjin Synthetic Biotechnology Innovation Capacity Improvement Project[TSBICIP-KJGG-003]
WOS Research AreaChemistry
WOS SubjectChemistry, Multidisciplinary
Funding OrganizationNational Key Research and Development Program of China ; National Natural Science Funds of China ; Natural Science Fund of Tianjin ; Open Funding Project of the State Key Laboratory of Biochemical Engineering ; Tianjin Synthetic Biotechnology Innovation Capacity Improvement Project
WOS IDWOS:000714412200001
PublisherROYAL SOC CHEMISTRY
Citation statistics
Document Type期刊论文
Identifierhttp://ir.ipe.ac.cn/handle/122111/50888
Collection中国科学院过程工程研究所
Corresponding AuthorShi, Jiafu; Jiang, Zhongyi
Affiliation1.Tianjin Univ, Sch Environm Sci & Engn, Tianjin 300072, Peoples R China
2.Tianjin Univ, Sch Chem Engn & Technol, Key Lab Green Chem Technol, Minist Educ, Tianjin 300072, Peoples R China
3.Collaborat Innovat Ctr Chem Sci & Engn Tianjin, Tianjin 300072, Peoples R China
4.Tianjin Univ, Joint Sch Natl Univ Singapore & Tianjin Univ, Int Campus, Fuzhou 350207, Peoples R China
5.Chinese Acad Sci, State Key Lab Biochem Engn, Inst Proc Engn, Beijing 10090, Peoples R China
6.Radboud Univ Nijmegen, Inst Mol & Mat, Nijmegen, Netherlands
Recommended Citation
GB/T 7714
Zhang, Shaohua,Liu, Shusong,Sun, Yiying,et al. Enzyme-photo-coupled catalytic systems[J]. CHEMICAL SOCIETY REVIEWS,2021:18.
APA Zhang, Shaohua,Liu, Shusong,Sun, Yiying,Li, Shihao,Shi, Jiafu,&Jiang, Zhongyi.(2021).Enzyme-photo-coupled catalytic systems.CHEMICAL SOCIETY REVIEWS,18.
MLA Zhang, Shaohua,et al."Enzyme-photo-coupled catalytic systems".CHEMICAL SOCIETY REVIEWS (2021):18.
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