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A Review on the Design and Performance of Enzyme-Aided Catalysis of Carbon Dioxide in Membrane, Electrochemical Cell and Photocatalytic Reactors
Ahmad Rizal Lim, Fatin Nasreen1; Marpani, Fauziah1,2; Anak Dilol, Victoria Eliz1; Mohamad Pauzi, Syazana1; Othman, Nur Hidayati1; Alias, Nur Hashimah1,2; Nik Him, Nik Raikhan1,2; Luo, Jianquan3; Abd Rahman, Norazah1
2022
Source PublicationMEMBRANES
Volume12Issue:1Pages:28
AbstractMulti-enzyme cascade catalysis involved three types of dehydrogenase enzymes, namely, formate dehydrogenase (FDH), formaldehyde dehydrogenase (FaldDH), alcohol dehydrogenase (ADH), and an equimolar electron donor, nicotinamide adenine dinucleotide (NADH), assisting the reaction is an interesting pathway to reduce thermodynamically stable molecules of CO2 from the atmosphere. The biocatalytic sequence is interesting because it operates under mild reaction conditions (low temperature and pressure) and all the enzymes are highly selective, which allows the reaction to produce three basic chemicals (formic acid, formaldehyde, and methanol) in just one pot. There are various challenges, however, in applying the enzymatic conversion of CO2, namely, to obtain high productivity, increase reusability of the enzymes and cofactors, and to design a simple, facile, and efficient reactor setup that will sustain the multi-enzymatic cascade catalysis. This review reports on enzyme-aided reactor systems that support the reduction of CO2 to methanol. Such systems include enzyme membrane reactors, electrochemical cells, and photocatalytic reactor systems. Existing reactor setups are described, product yields and biocatalytic productivities are evaluated, and effective enzyme immobilization methods are discussed.
Keywordenzyme membrane reactor enzyme immobilization carbon dioxide reduction photocatalytic electrochemical
DOI10.3390/membranes12010028
Language英语
WOS KeywordFORMATE DEHYDROGENASE ; CO2 REDUCTION ; RECENT PROGRESS ; EFFICIENT CONVERSION ; METHANOL ; IMMOBILIZATION ; GRAPHENE ; REGENERATION ; FORMALDEHYDE ; SYSTEM
Funding ProjectMinistry of Higher Education, Malaysia under the Fundamental Research Grant Scheme[FRGS/1/2019/TK02/UITM/03/5]
WOS Research AreaBiochemistry & Molecular Biology ; Chemistry ; Engineering ; Materials Science ; Polymer Science
WOS SubjectBiochemistry & Molecular Biology ; Chemistry, Physical ; Engineering, Chemical ; Materials Science, Multidisciplinary ; Polymer Science
Funding OrganizationMinistry of Higher Education, Malaysia under the Fundamental Research Grant Scheme
WOS IDWOS:000750551100001
PublisherMDPI
Citation statistics
Document Type期刊论文
Identifierhttp://ir.ipe.ac.cn/handle/122111/51912
Collection中国科学院过程工程研究所
Corresponding AuthorMarpani, Fauziah
Affiliation1.Univ Teknol MARA, Coll Engn, Sch Chem Engn, Shah Alam 40450, Malaysia
2.Univ Teknol MARA, Coll Engn, Sch Chem Engn, Catalysis Sustainable Water & Energy Nexus Res Gr, Shah Alam 40450, Malaysia
3.Chinese Acad Sci, Inst Proc Engn, State Key Lab Biochem Engn, Beijing 100190, Peoples R China
Recommended Citation
GB/T 7714
Ahmad Rizal Lim, Fatin Nasreen,Marpani, Fauziah,Anak Dilol, Victoria Eliz,et al. A Review on the Design and Performance of Enzyme-Aided Catalysis of Carbon Dioxide in Membrane, Electrochemical Cell and Photocatalytic Reactors[J]. MEMBRANES,2022,12(1):28.
APA Ahmad Rizal Lim, Fatin Nasreen.,Marpani, Fauziah.,Anak Dilol, Victoria Eliz.,Mohamad Pauzi, Syazana.,Othman, Nur Hidayati.,...&Abd Rahman, Norazah.(2022).A Review on the Design and Performance of Enzyme-Aided Catalysis of Carbon Dioxide in Membrane, Electrochemical Cell and Photocatalytic Reactors.MEMBRANES,12(1),28.
MLA Ahmad Rizal Lim, Fatin Nasreen,et al."A Review on the Design and Performance of Enzyme-Aided Catalysis of Carbon Dioxide in Membrane, Electrochemical Cell and Photocatalytic Reactors".MEMBRANES 12.1(2022):28.
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