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Rotten Eggs Revaluated: Ionic Liquids and Deep Eutectic Solvents for Removal and Utilization of Hydrogen Sulfide
Li, Fangfang3; Laaksonen, Aatto3,4,5,6; Zhang, Xiangping1,2; Ji, Xiaoyan3
2022-02-23
Source PublicationINDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
ISSN0888-5885
Volume61Issue:7Pages:2643-2671
AbstractHydrogen sulfide (H2S) is highly toxic and one of the problematic impurities in industrial gas streams, calling for H2S removal down to single-digit ppm levels to protect health and environment, and not to harm to the downstream processes. Here, we discuss the recent developments and challenges of current H2S removal technologies. Furthermore, we present a comprehensive review of H2S removal in ionic liquids (ILs), IL-based solvents/adsorbents/membranes, and deep eutectic solvents (DESs) due to their unique advantages. We analyze theoretical studies to better understand the microscopic details behind H2S removal. We discuss new research on IL/DES-based H2S removal processes from an industrial perspective. Finally, we summarize the utilization of H2S in IL/DES-based systems for the recovery of sulfur and hydrogen, and synthesis of value-added chemicals. This review will provide both general and in-depth knowledge of the achievements, difficulties, and research priorities in developing novel ILs/DESs for efficient and sustainable H2S removal and utilization.
DOI10.1021/acs.iecr.1c04142
Language英语
WOS KeywordGROUP-CONTRIBUTION EQUATION ; HIGHLY EFFICIENT CAPTURE ; ACID GASES SOLUBILITY ; PC-SAFT EQUATIONS ; ROOM-TEMPERATURE ; H2S SOLUBILITY ; OF-STATE ; DESULFURIZATION PERFORMANCE ; CARBON-DIOXIDE ; BINARY-MIXTURES
Funding ProjectSwedish Energy Agency[P47500-1] ; Swedish Research Council ; Ministry of Research and Innovation of Romania (CNCS-UEFISCDI) within PNCDI III[PN-III-P4-ID-PCCF-2016-0050]
WOS Research AreaEngineering
WOS SubjectEngineering, Chemical
Funding OrganizationSwedish Energy Agency ; Swedish Research Council ; Ministry of Research and Innovation of Romania (CNCS-UEFISCDI) within PNCDI III
WOS IDWOS:000766191300001
PublisherAMER CHEMICAL SOC
Citation statistics
Document Type期刊论文
Identifierhttp://ir.ipe.ac.cn/handle/122111/52265
Collection中国科学院过程工程研究所
Corresponding AuthorZhang, Xiangping; Ji, Xiaoyan
Affiliation1.Chinese Acad Sci, CAS Key Lab Green Proc & Engn, Beijing Key Lab Ion Liquids Clean Proc, State Key Lab Multiphase Complex Syst,Inst Proc E, Beijing 100190, Peoples R China
2.Univ Chinese Acad Sci, Sch Chem Engn, Beijing 100049, Peoples R China
3.Lulea Univ Technol, Div Energy Sci, Energy Engn, S-97187 Lulea, Sweden
4.Stockholm Univ, Dept Mat & Environm Chem, Arrhenius Lab, Div Phys Chem, S-10691 Stockholm, Sweden
5.Petru Poni Inst Macromol Chem, Ctr Adv Res Bionanoconjugates & Biopolymers, Iasi 700469, Romania
6.Nanjing Tech Univ, State Key Lab Mat Oriented & Chem Engn, Nanjing 211816, Peoples R China
Recommended Citation
GB/T 7714
Li, Fangfang,Laaksonen, Aatto,Zhang, Xiangping,et al. Rotten Eggs Revaluated: Ionic Liquids and Deep Eutectic Solvents for Removal and Utilization of Hydrogen Sulfide[J]. INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,2022,61(7):2643-2671.
APA Li, Fangfang,Laaksonen, Aatto,Zhang, Xiangping,&Ji, Xiaoyan.(2022).Rotten Eggs Revaluated: Ionic Liquids and Deep Eutectic Solvents for Removal and Utilization of Hydrogen Sulfide.INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,61(7),2643-2671.
MLA Li, Fangfang,et al."Rotten Eggs Revaluated: Ionic Liquids and Deep Eutectic Solvents for Removal and Utilization of Hydrogen Sulfide".INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH 61.7(2022):2643-2671.
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