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Aerobic Oxidation of Benzyl Alcohol over Activated Carbon Supported Manganese and Vanadium Catalysts: Effect of Surface Oxygen-Containing Groups
Chen, Yuanting1; Chen, Wan1; Tang, Qinghu1; Guo, Zhen1; Yang, Yanhui1; Su, Fabing2; Yang, YH
2011
Source PublicationCATALYSIS LETTERS
ISSN1011-372X
Volume141Issue:1Pages:149-157
AbstractIn this contribution, the selective oxidation of benzyl alcohol using molecular oxygen over supported manganese and vanadium catalysts was investigated. The catalytic activities were significantly improved after pre-oxidizing the activated carbon support materials. Characterizations of nitrogen physisorption, X-ray diffraction, transmission electron microscopy, and X-ray absorption were involved to examine the physicochemical properties of as-prepared catalysts. By ruling out the effects of specific surface area, active site dispersion, valence and local coordination of Mn and V active species, the improved catalytic activity was attributed to the specific variety and increased density of oxygen-containing groups on activated carbon support surfaces, which was further confirmed by cyclic voltammetry measurements and Fourier transform infrared spectroscopy.
KeywordActivated Carbon Surface Oxygen Manganese Oxides Vanadium Oxides Benzyl Alcohol Oxidation
SubtypeArticle
WOS HeadingsScience & Technology ; Physical Sciences
DOI10.1007/s10562-010-0447-4
Indexed BySCI
Language英语
WOS KeywordABSORPTION FINE-STRUCTURE ; SELECTIVE OXIDATION ; RUTHENIUM CATALYSTS ; AROMATIC ALCOHOLS ; PLATINUM ; CINNAMALDEHYDE ; HYDROGENATION ; CHEMISTRY ; PERFORMANCE ; EPOXIDATION
WOS Research AreaChemistry
WOS SubjectChemistry, Physical
WOS IDWOS:000286380900019
Citation statistics
Cited Times:14[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Version出版稿
Identifierhttp://ir.ipe.ac.cn/handle/122111/5258
Collection多相复杂系统国家重点实验室
Corresponding AuthorYang, YH
Affiliation1.Nanyang Technol Univ, Sch Chem & Biomed Engn, Singapore 637459, Singapore
2.Chinese Acad Sci, State Key Lab Multiphase Complex Syst, Inst Proc Engn, Beijing 100190, Peoples R China
Recommended Citation
GB/T 7714
Chen, Yuanting,Chen, Wan,Tang, Qinghu,et al. Aerobic Oxidation of Benzyl Alcohol over Activated Carbon Supported Manganese and Vanadium Catalysts: Effect of Surface Oxygen-Containing Groups[J]. CATALYSIS LETTERS,2011,141(1):149-157.
APA Chen, Yuanting.,Chen, Wan.,Tang, Qinghu.,Guo, Zhen.,Yang, Yanhui.,...&Yang, YH.(2011).Aerobic Oxidation of Benzyl Alcohol over Activated Carbon Supported Manganese and Vanadium Catalysts: Effect of Surface Oxygen-Containing Groups.CATALYSIS LETTERS,141(1),149-157.
MLA Chen, Yuanting,et al."Aerobic Oxidation of Benzyl Alcohol over Activated Carbon Supported Manganese and Vanadium Catalysts: Effect of Surface Oxygen-Containing Groups".CATALYSIS LETTERS 141.1(2011):149-157.
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