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Vertically Heterostructured Solid Electrolytes for Lithium Metal Batteries
He, Fei1; Hu, Zhenglin1; Tang, Wenjing1; Wang, Aoxuan1; Wen, Bohua2; Zhang, Lan3; Luo, Jiayan1,4
2022-04-12
Source PublicationADVANCED FUNCTIONAL MATERIALS
ISSN1616-301X
Pages23
AbstractSolid-state electrolytes (SSEs) have been regarded as the most attractive candidate for safe and high-energy lithium (Li) batteries of the next generation. However, the inability of current SSEs to keep up with the performance requirements of batteries is significantly affected by complex factors, especially ionic conductivity, mechanochemical properties, and coupled ion/electron reaction at the electrified interfaces. Strategies in solid electrolyte chemistries and technologies are put forward to overcome these challenges while widening the breadth of possible applications. Among them, vertically heterostructured solid-state electrolytes (HSE) are constructed as a most promising strategy, which can take advantage of individual SSE layers together and rationalize the stability and compatibility of electrodes. This review comprehensively summarizes the specific features of the HSE based on the current knowledge of SSE failure modes. Additionally, a detailed review of the recent progress on the HSE design in terms of organic polymer electrolytes and inorganic electrolytes is generated. Finally, the advantages and drawbacks of the design strategies are discussed. New perspectives about HSE are proposed as well.
Keywordinterphases lithium metal anodes mechanisms solid electrolytes stability
DOI10.1002/adfm.202201465
Language英语
WOS KeywordLI-ION CONDUCTIVITY ; POLYMER ELECTROLYTES ; INTERFACE STABILITY ; COMPOSITE ELECTROLYTES ; INTERPHASE FORMATION ; MECHANICAL CONSTRICTION ; POLY(ETHYLENE OXIDE) ; STATE ELECTROLYTES ; GRAIN-BOUNDARIES ; LAYER FORMATION
Funding ProjectNational Key Research and Development Program of China[2021YFB2500100] ; National Natural Science Foundation of China[51872196]
WOS Research AreaChemistry ; Science & Technology - Other Topics ; Materials Science ; Physics
WOS SubjectChemistry, Multidisciplinary ; Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter
Funding OrganizationNational Key Research and Development Program of China ; National Natural Science Foundation of China
WOS IDWOS:000781631700001
PublisherWILEY-V C H VERLAG GMBH
Citation statistics
Document Type期刊论文
Identifierhttp://ir.ipe.ac.cn/handle/122111/52614
Collection中国科学院过程工程研究所
Corresponding AuthorWang, Aoxuan; Luo, Jiayan
Affiliation1.Tianjin Univ, Sch Chem Engn & Technol, Key Lab Green Chem Technol, Minist Educ, Tianjin 300072, Peoples R China
2.Tsinghua Univ, Shenzhen Int Grad Sch, Shenzhen 518055, Peoples R China
3.Chinese Acad Sci, CAS Key Lab Green Proc & Engn, Beijing Key Lab Ion Liquids Clean Proc, State Key Lab Multiphase Complex Syst,Inst Proc E, Beijing 100190, Peoples R China
4.Shanghai Jiao Tong Univ, Sch Mat Sci & Engn, Shanghai Key Lab Adv High Temp Mat & Precis Formi, Shanghai 200240, Peoples R China
Recommended Citation
GB/T 7714
He, Fei,Hu, Zhenglin,Tang, Wenjing,et al. Vertically Heterostructured Solid Electrolytes for Lithium Metal Batteries[J]. ADVANCED FUNCTIONAL MATERIALS,2022:23.
APA He, Fei.,Hu, Zhenglin.,Tang, Wenjing.,Wang, Aoxuan.,Wen, Bohua.,...&Luo, Jiayan.(2022).Vertically Heterostructured Solid Electrolytes for Lithium Metal Batteries.ADVANCED FUNCTIONAL MATERIALS,23.
MLA He, Fei,et al."Vertically Heterostructured Solid Electrolytes for Lithium Metal Batteries".ADVANCED FUNCTIONAL MATERIALS (2022):23.
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