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| Vertically Heterostructured Solid Electrolytes for Lithium Metal Batteries | |
| He, Fei1; Hu, Zhenglin1; Tang, Wenjing1; Wang, Aoxuan1; Wen, Bohua2; Zhang, Lan3; Luo, Jiayan1,4 | |
| 2022-04-12 | |
| Source Publication | ADVANCED FUNCTIONAL MATERIALS
 |
| ISSN | 1616-301X |
| Pages | 23 |
| Abstract | Solid-state electrolytes (SSEs) have been regarded as the most attractive candidate for safe and high-energy lithium (Li) batteries of the next generation. However, the inability of current SSEs to keep up with the performance requirements of batteries is significantly affected by complex factors, especially ionic conductivity, mechanochemical properties, and coupled ion/electron reaction at the electrified interfaces. Strategies in solid electrolyte chemistries and technologies are put forward to overcome these challenges while widening the breadth of possible applications. Among them, vertically heterostructured solid-state electrolytes (HSE) are constructed as a most promising strategy, which can take advantage of individual SSE layers together and rationalize the stability and compatibility of electrodes. This review comprehensively summarizes the specific features of the HSE based on the current knowledge of SSE failure modes. Additionally, a detailed review of the recent progress on the HSE design in terms of organic polymer electrolytes and inorganic electrolytes is generated. Finally, the advantages and drawbacks of the design strategies are discussed. New perspectives about HSE are proposed as well. |
| Keyword | interphases lithium metal anodes mechanisms solid electrolytes stability |
| DOI | 10.1002/adfm.202201465 |
| Language | 英语 |
| WOS Keyword | LI-ION CONDUCTIVITY ; POLYMER ELECTROLYTES ; INTERFACE STABILITY ; COMPOSITE ELECTROLYTES ; INTERPHASE FORMATION ; MECHANICAL CONSTRICTION ; POLY(ETHYLENE OXIDE) ; STATE ELECTROLYTES ; GRAIN-BOUNDARIES ; LAYER FORMATION |
| Funding Project | National Key Research and Development Program of China[2021YFB2500100] ; National Natural Science Foundation of China[51872196] |
| WOS Research Area | Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics |
| WOS Subject | Chemistry, Multidisciplinary ; Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter |
| Funding Organization | National Key Research and Development Program of China ; National Natural Science Foundation of China |
| WOS ID | WOS:000781631700001 |
| Publisher | WILEY-V C H VERLAG GMBH |
| Citation statistics | |
| Document Type | 期刊论文 |
| Identifier | http://ir.ipe.ac.cn/handle/122111/52614 |
| Collection | 中国科学院过程工程研究所 |
| Corresponding Author | Wang, Aoxuan; Luo, Jiayan |
| Affiliation | 1.Tianjin Univ, Sch Chem Engn & Technol, Key Lab Green Chem Technol, Minist Educ, Tianjin 300072, Peoples R China 2.Tsinghua Univ, Shenzhen Int Grad Sch, Shenzhen 518055, Peoples R China 3.Chinese Acad Sci, CAS Key Lab Green Proc & Engn, Beijing Key Lab Ion Liquids Clean Proc, State Key Lab Multiphase Complex Syst,Inst Proc E, Beijing 100190, Peoples R China 4.Shanghai Jiao Tong Univ, Sch Mat Sci & Engn, Shanghai Key Lab Adv High Temp Mat & Precis Formi, Shanghai 200240, Peoples R China |
| Recommended Citation GB/T 7714 | He, Fei,Hu, Zhenglin,Tang, Wenjing,et al. Vertically Heterostructured Solid Electrolytes for Lithium Metal Batteries[J]. ADVANCED FUNCTIONAL MATERIALS,2022:23. |
| APA | He, Fei.,Hu, Zhenglin.,Tang, Wenjing.,Wang, Aoxuan.,Wen, Bohua.,...&Luo, Jiayan.(2022).Vertically Heterostructured Solid Electrolytes for Lithium Metal Batteries.ADVANCED FUNCTIONAL MATERIALS,23. |
| MLA | He, Fei,et al."Vertically Heterostructured Solid Electrolytes for Lithium Metal Batteries".ADVANCED FUNCTIONAL MATERIALS (2022):23. |
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