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| Electrocatalytic Reduction of Nitrogen to Ammonia in Ionic Liquids br | |
| Tian, Yuan1,2; Liu, Yanrong2,3; Wang, Hao2; Liu, Lei2,4; Hu, Wenping1 | |
| 2022-04-11 | |
| Source Publication | ACS SUSTAINABLE CHEMISTRY & ENGINEERING
 |
| ISSN | 2168-0485 |
| Volume | 10Issue:14Pages:4345-4358 |
| Abstract | Ammonia (NH3) is an important raw material fornitrogen fertilizer production and is widely used in industry. It is alsoa carbon-free renewable fuel and an excellent hydrogen storagematerial. Reaction conditions of the traditional Haber-Bosch processare very harsh even though it supports most of today'sNH3production. Recently, the electrocatalytic nitrogen reduction reaction(NRR) has become one of the effective alternative methods to thetraditional Haber-Bosch process due to the advantages of mildoperation conditions and almost no environmental pollution. Ionicliquids (ILs) act as one of the green solvents that possess a lot ofunique features and have shown excellent performance in theelectrocatalytic NRR process. In this perspective, we summarize thefundamentals of the electrocatalytic NRR, the role of ILs in severaltypical electrocatalytic processes, and the possible role of ILs in theelectrocatalytic NRR process. Moreover, the selection principles and issues of the application of ILs as well as the futuredevelopment directions for the electrocatalytic NRR process are presented. |
| Keyword | Ammonia synthesis Electrocatalysis Nitrogen reduction reaction Ionic liquids Electrocatalytic NRR process Ambient conditions |
| DOI | 10.1021/acssuschemeng.2c00018 |
| Language | 英语 |
| WOS Keyword | ELECTROCHEMICAL REDUCTION ; OXYGEN-REDUCTION ; PHYSICOCHEMICAL PROPERTIES ; CARBON-DIOXIDE ; CO2 REDUCTION ; CATALYSTS ; N-2 ; SOLUBILITY ; DINITROGEN ; CONVERSION |
| WOS Research Area | Chemistry ; Science & Technology - Other Topics ; Engineering |
| WOS Subject | Chemistry, Multidisciplinary ; Green & Sustainable Science & Technology ; Engineering, Chemical |
| WOS ID | WOS:000791025300002 |
| Publisher | AMER CHEMICAL SOC |
| Citation statistics | |
| Document Type | 期刊论文 |
| Identifier | http://ir.ipe.ac.cn/handle/122111/53348 |
| Collection | 中国科学院过程工程研究所 |
| Corresponding Author | Liu, Lei; Hu, Wenping |
| Affiliation | 1.Tianjin Univ, Sch Sci, Dept Chem, Tianjin Key Lab Mol Optoelect Sci, Tianjin 300072, Peoples R China 2.Chinese Acad Sci, Beijing Key Lab Ion Liquids Clean Proc, CAS Key Lab Green Proc & Engn, State Key Lab Multiphase Complex Syst,Inst Proc E, Beijing 100190, Peoples R China 3.Zhengzhou Inst Emerging Ind Technol, Zhengzhou 450000, Peoples R China 4.Wuhan Text Univ, Sch Chem & Chem Engn, Wuhan 430200, Peoples R China |
| Recommended Citation GB/T 7714 | Tian, Yuan,Liu, Yanrong,Wang, Hao,et al. Electrocatalytic Reduction of Nitrogen to Ammonia in Ionic Liquids br[J]. ACS SUSTAINABLE CHEMISTRY & ENGINEERING,2022,10(14):4345-4358. |
| APA | Tian, Yuan,Liu, Yanrong,Wang, Hao,Liu, Lei,&Hu, Wenping.(2022).Electrocatalytic Reduction of Nitrogen to Ammonia in Ionic Liquids br.ACS SUSTAINABLE CHEMISTRY & ENGINEERING,10(14),4345-4358. |
| MLA | Tian, Yuan,et al."Electrocatalytic Reduction of Nitrogen to Ammonia in Ionic Liquids br".ACS SUSTAINABLE CHEMISTRY & ENGINEERING 10.14(2022):4345-4358. |
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