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In situ complex coacervation supported by self-coated polydopamine interlayer on uniform-sized essential oils droplet
Tian, Qirui1,2; Zhou, Weiqing2,3; Cai, Qiong1; Pan, Xiaoyun4; Ma, Guanghui2,3; Lian, Guoping1,5
2022-10-01
Source PublicationJOURNAL OF COLLOID AND INTERFACE SCIENCE
ISSN0021-9797
Volume623Pages:1027-1038
AbstractHypothesis: Essential oils (EOs) are common additives in daily products by virtue of their olfactory, physicochemical, and biological characteristics. However, EOs are physicochemically unstable and susceptible to degradation or loss, leading to limited shelf life and inadequate efficacy. Herein we propose a new bi-layered encapsulation structure in combination with complex coacervation and self-coating of polydopamine (PDA) on membrane emulsified mono-dispersion of EOs droplets.Experiments: A mono-dispersed EOs emulsion stabilized by nonionic surfactants was produced by membrane emulsification, wherein the EOs droplets were applied as soft templates to deposit a superficial PDA layer. Under alkaline conditions, gelatin (GE) was bound to the PDA layer and further applied as in situ coacervation sites for gum Arabic (GA). Structural identification and morphological observation proved the successful preparation of bi-layered EOs capsules.Findings: Compared with traditional complex coacervation strategies, current novel bi-layered capsules showed significantly improved structural stability, thermal stability, providing better protection of EOs with sustained release properties. Moreover, the encapsulation efficiency and loading content were both proved higher for the bi-layered system. The first report on PDA-coating onto surfactants-absorbed macroemulsion droplets also provides an in-depth insight into applying PDA as versatile intermediate functional biomaterials.(c) 2022 Elsevier Inc. All rights reserved.
KeywordEssential oils Polydopamine Shell functionalization Complex coacervation Membrane emulsification Bi-layered capsule Sustained release
DOI10.1016/j.jcis.2022.05.072
Language英语
WOS KeywordEMULSION ; MICROCAPSULES ; GELATIN ; STABILITY ; SURFACE ; DEPOSITION ; MICROENCAPSULATION ; NANOPARTICLES ; ENCAPSULATION ; DOPAMINE
Funding ProjectNational Key Research and Development Program of China[2020YFA0112603] ; Strategic Priority Research Program of the Chinese Academy of Sciences[XDA16020405] ; Ministry of Science and Technology of China[21821005] ; University of Surrey (UK) ; Unilever (UK) ; Institute of Process Engineering (China)
WOS Research AreaChemistry
WOS SubjectChemistry, Physical
Funding OrganizationNational Key Research and Development Program of China ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Ministry of Science and Technology of China ; University of Surrey (UK) ; Unilever (UK) ; Institute of Process Engineering (China)
WOS IDWOS:000810421700008
PublisherACADEMIC PRESS INC ELSEVIER SCIENCE
Citation statistics
Document Type期刊论文
Identifierhttp://ir.ipe.ac.cn/handle/122111/53976
Collection中国科学院过程工程研究所
Corresponding AuthorZhou, Weiqing; Ma, Guanghui; Lian, Guoping
Affiliation1.Univ Surrey, Dept Chem & Proc Engn, Guildford GU2 7XH, Surrey, England
2.Chinese Acad Sci, Inst Proc Engn, State Key Lab Biochem Engn, Beijing 100190, Peoples R China
3.Univ Chinese Acad Sci, Sch Chem Sci, Beijing 100049, Peoples R China
4.Unilever Res & Dev Shanghai Ctr, 66 Lin Xin Rd, Shanghai 200335, Peoples R China
5.Unilever Res Colworth, Colworth Pk, Sharnbrook MK44 1LQ, Bedfordshire, England
Recommended Citation
GB/T 7714
Tian, Qirui,Zhou, Weiqing,Cai, Qiong,et al. In situ complex coacervation supported by self-coated polydopamine interlayer on uniform-sized essential oils droplet[J]. JOURNAL OF COLLOID AND INTERFACE SCIENCE,2022,623:1027-1038.
APA Tian, Qirui,Zhou, Weiqing,Cai, Qiong,Pan, Xiaoyun,Ma, Guanghui,&Lian, Guoping.(2022).In situ complex coacervation supported by self-coated polydopamine interlayer on uniform-sized essential oils droplet.JOURNAL OF COLLOID AND INTERFACE SCIENCE,623,1027-1038.
MLA Tian, Qirui,et al."In situ complex coacervation supported by self-coated polydopamine interlayer on uniform-sized essential oils droplet".JOURNAL OF COLLOID AND INTERFACE SCIENCE 623(2022):1027-1038.
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