CAS OpenIR
Impact of cooking style and oil on semi-volatile and intermediate volatility organic compound emissions from Chinese domestic cooking
Song, Kai1,2; Guo, Song1,2; Gong, Yuanzheng1; Lv, Daqi1; Zhang, Yuan1,3; Wan, Zichao1; Li, Tianyu1; Zhu, Wenfei1; Wang, Hui1; Yu, Ying; Tan, Rui; Shen, Ruizhe1; Lu, Sihua1; Li, Shuangde4; Chen, Yunfa4; Hu, Min1,2
2022-08-02
Source PublicationATMOSPHERIC CHEMISTRY AND PHYSICS
ISSN1680-7316
Volume22Issue:15Pages:9827-9841
AbstractTo elucidate the molecular chemical compositions, volatility-polarity distributions, and influencing factors of Chinese cooking emissions, a comprehensive cooking emission experiment was conducted. Volatile organic compounds (VOCs), intermediate volatility, and semi-volatile organic compounds (I/SVOCs) from cooking fumes were analysed by a thermal desorption comprehensive two-dimensional gas chromatography coupled with quadrupole mass spectrometer (TD-GC x GC-qMS). Emissions from four typical Chinese dishes, i.e. fried chicken, Kung Pao chicken, pan-fried tofu, and stir-fried cabbage were investigated to illustrate the impact of cooking style and material. Fumes of chicken fried with corn, peanut, soybean, and sunflower oils were investigated to demonstrate the influence of cooking oil. A total of 201 chemicals were quantified. Kung Pao chicken emitted more pollutants than other dishes due to its rather intense cooking method. Aromatics and oxygenated compounds were extensively detected among meat-related cooking fumes, while a vegetable-related profile was observed in the emissions of stir-fried cabbage. Ozone formation potential (OFP) was dominated by chemicals in the VOC range. Of the secondary organic aerosol (SOA) estimation, 10.2 %-32.0 % could be explained by S/IVOCs. Pixel-based partial least squares discriminant analysis (PLS-DA) and multiway principal component analysis (MPCA) were utilized for sample classification and component identification. The results indicated that the oil factor explained more variance of chemical compositions than the cooking style factor. MPCA results emphasize the importance of the unsaturated fatty acid-alkadienal-volatile products mechanism (oil autoxidation) accelerated by the cooking and heating procedure.
DOI10.5194/acp-22-9827-2022
Language英语
WOS KeywordRADICAL-INITIATED REACTIONS ; AROMATIC-HYDROCARBONS PAHS ; HEALTH-RISK ASSESSMENT ; AIR-POLLUTION SOURCES ; AEROSOL FORMATION ; PARTICULATE MATTER ; CHEMICAL CHARACTERISTICS ; MOLECULAR-STRUCTURE ; VEGETABLE-OILS ; BASIS-SET
Funding ProjectNational Natural Science Foundation of China[41977179] ; National Natural Science Foundation of China[91844301] ; State Key Joint Laboratory of Environmental Simulation and Pollution Control[22Y01SSPCP] ; State Key Laboratory of Multi-phase Complex Systems[MPCS-2021-D-12]
WOS Research AreaEnvironmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
WOS SubjectEnvironmental Sciences ; Meteorology & Atmospheric Sciences
Funding OrganizationNational Natural Science Foundation of China ; State Key Joint Laboratory of Environmental Simulation and Pollution Control ; State Key Laboratory of Multi-phase Complex Systems
WOS IDWOS:000834829900001
PublisherCOPERNICUS GESELLSCHAFT MBH
Citation statistics
Document Type期刊论文
Identifierhttp://ir.ipe.ac.cn/handle/122111/54345
Collection中国科学院过程工程研究所
Corresponding AuthorGuo, Song
Affiliation1.Coll Environm Sci & Engn, State Key Joint Lab Environm Simulat & Pollut Con, Int Joint Lab Reg Pollut Control, Minist Educ IJRC, Beijing 100871, Peoples R China
2.Nanjing Univ Informat Sci Technol, Collaborat Innovat Ctr Atmospher Environm & Equip, Nanjing 210044, Peoples R China
3.Hebei Univ Engn, Sch Earth Sci & Engn, Handan 056038, Peoples R China
4.Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China
Recommended Citation
GB/T 7714
Song, Kai,Guo, Song,Gong, Yuanzheng,et al. Impact of cooking style and oil on semi-volatile and intermediate volatility organic compound emissions from Chinese domestic cooking[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2022,22(15):9827-9841.
APA Song, Kai.,Guo, Song.,Gong, Yuanzheng.,Lv, Daqi.,Zhang, Yuan.,...&Hu, Min.(2022).Impact of cooking style and oil on semi-volatile and intermediate volatility organic compound emissions from Chinese domestic cooking.ATMOSPHERIC CHEMISTRY AND PHYSICS,22(15),9827-9841.
MLA Song, Kai,et al."Impact of cooking style and oil on semi-volatile and intermediate volatility organic compound emissions from Chinese domestic cooking".ATMOSPHERIC CHEMISTRY AND PHYSICS 22.15(2022):9827-9841.
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